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Quantum-based spectroscopy and efficient energy transport with biomolecules

  • Autores: Roberto de Jesús León Montiel
  • Directores de la Tesis: Juan Pérez Torres (dir. tes.)
  • Lectura: En la Universitat Politècnica de Catalunya (UPC) ( España ) en 2014
  • Idioma: inglés
  • Tribunal Calificador de la Tesis: Jordi Mompart (presid.), Hugues de Riedmatten (secret.), Jan Perina (voc.)
  • Materias:
  • Enlaces
    • Tesis en acceso abierto en: TDX
  • Resumen
    • For many years, the fields of quantum optics and biology have rarely shared a common path. In quantum optics, most of the concepts and techniques developed over the years stand for systems where only a few degrees of freedom are considered and, more importantly, where the systems under study are assumed to be completely isolated from their surrounding environment. This situation is far from what we can find in nature. Biological complexes are, by definition, warm, wet and noisy systems subjected to environmental fluctuations, where quantum phenomena are unlikely to be observed. Notwithstanding, in recent years, this paradigm has begun to be questioned by several works where quantum-mechanical concepts have been introduced in order to describe the dynamics of important biological processes, such as energy transport in photosynthetic light-harvesting complexes. The goal of this thesis is twofold. Firstly, we will investigate how ideas and techniques routinely used in quantum optics can be exploited in order to develop new quantum-based spectroscopy techniques and, secondly, we will examine to what extent microscopic quantum phenomena could impact on the efficient transport behavior of photosynthetic light-havesting complexes. This problem is particularly relevant, because the understanding of the fundamental mechanisms that enable the highly efficient transport of energy in photosynthetic systems could lead us to the design of future quantum-inspired light-harvesting technologies, such as high-efficiency organic solar cells.


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